Library Creation

Recently we were discussing about creating a book through Accessible Horizon Films, sort of a learning tool for the kids at Siragu Montessori School. In fact, we were even thinking of building a library source for them. Although this is in the very basic stages of development, we need ideas on what topics to cover. We suggested comic books like Amar Chitra Katha, Tinkle, Archies, etc which are an effective way towards cognitive development in English, the language and its grammar. There is no specific genre of books or topics you can suggest, just that we have to be creative to pick topics/books that can help in overall development of children aged 3-10. So if anyone has any ideas, please feel free to share them with us.
The goal: Create a library of books, resources for Siragu School, so by the end of a year, they will have something to go to, for creative/knowledge acquisition.